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Bo A's second Japanese studio album, Valenti (2003), became her best-selling album, with over 1,249,000 copies sold.
Later that year, she released two Korean albums, Atlantis Princess and the mini-album Shine We Are! The former was the fifth-best-selling South Korean record of the year with around 345,000 units sold; the latter sold around 58,000 units.
Bo A released two more singles "Kiseki / No.1" and "Jewel Song / Beside You: Boku o Yobu Koe", both which also peaked at the number-three position.
In contrast with 1st Live Tour, which "emphasized exotic Asian design", the Love & Honesty tour had an "outer-space, sci-fi" theme; among the props were a three-story-high space ship and the robot Asimo.The tour, which lasted until October 29, started from Nagoya and contained twelve shows, two in each of the following cities: Nagoya, Fukuoka, Osaka, Tokyo, Sendai, and Sapporo.She staged her first Christmas concert on December 7, 2006.On September 21, 2006, she released her first digital single in Korea, a Korean version of "Key of Heart".In support of Outgrow, Bo A launched a special Zepp tour, B0A The Live, on September 29, 2006.
Bo A's fifth Japanese studio album, Made in Twenty (2007), continued her transition from a "teenage girl" image to a more mature image.